Abstract
The ν 1 and ν 3 fundamental bands of 14NH 3 have been measured using the techniques of Fourier transform and coherent anti-Stokes Raman spectroscopy. The effective values of the band origins, rotational and centrifugal distortion constants, and parameters of the vibrational-rotational interactions have been obtained by analyzing these bands as essentially regular parallel and perpendicular bands, with the “off-diagonal” local resonance interactions excluded from the fit. The “diagonal” l-type resonance effects have been included into the analysis of the ν 3 band for the + l, K = 1 and − l, K = 2 levels.
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