Abstract
A theoretical model of donor–acceptor kinetics in the presence of energy migration and forward and reverse energy transfer taking into account correlations between molecules in the solution is presented. The model has been developed on the base of Markoffian and non-Markoffian theory of energy transfer recently proposed by Gochanour, Andersen and Fayer [J. Chem. Phys. 70, 4254 (1979)] and Loring, Andersen and Fayer [J. Chem. Phys. 76, 2015 (1982)]. It has been shown that correlations are an important factor in the case of forward and reverse energy transfer. This non-Markoffian behavior can be investigated experimentally.
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