Abstract
Formation of NH(A 3Π i ) has been studied in the photolysis of HN 3 at 121.6 nm. Measurements of time-resolved fluorescence intensity show that NH(A 3Π i ) is largely formed by secondary reactions involving two energetic intermediates which have lifetimes of 2.7 and 18 μs. These intermediates are tentatively assigned to N 2(B 3Π g, υ′) and N 2(B′ 3Σ u −), respectively.
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