Abstract
When 1,2-, 1,3-and 1,6-dimethylnaphthalene are oxidized by Ce 4+ in acetic acid the corresponding monoaldehydes are formed in better than 80% yield. In each case aldehyde formation takes place with a high degree of selectivity as the methyl-1- to methyl-2-naphthaldehyde ratio is better than 11:1. The selectivity may be explained from differences in reactivity as calculated within the frontier orbital method.
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