Abstract
Ion-molecule reactions occurring in Cr(CO) 6, Fe(CO) 5, and Mn 2(CO) 10 systems are carried out in a Fourier transform ion cyclotron resonance (FTICR) spectrometer. Abundant intensities of bare metal cluster ions can be formed by employing a multiple pulse sequence including selective ejections and photodissociation. In subsequent collisional activation experiments, the binding energies of Cr 2 + and Mn 2 + are determined as 1.6±0.2 and 2.1±0.3 eV, respectively, the latter being in conflict with a previously reported value.
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