Abstract
Pure YBa 2Cu 3O 7− δ (YBCO) and YBCO films with extended columnar defects comprised of self-assembled columns of nanodots and nanorods of BaZrO 3 (BZO), CaZrO 3 (CZO) and 8 mol.% Y 2O 3 stabilized ZrO 2 (YSZ) were prepared by pulsed laser deposition on RABiTS templates of configuration CeO 2/YSZ/Y 2O 3/Ni–W. Effects on increasing the size and density of columnar defects by varying the total volume fraction BZO, CZO or YSZ incorporations within the YBCO film are reported. BZO volume fraction was varied between 0% and 8%, CZO between 0% and 2% and YSZ 0–2%. The critical transition temperature ( T c) was found to linearly decrease with increase in vol.% of BZO, CZO and YSZ, with the steepest decline for CZO additions. Nevertheless, YBCO films with these columnar defects exhibit significantly reduced J c dependence on applied field. At 77 K, best properties are obtained for 1–2 vol.% BZO incorporation in the form of columns of self-assembled nanodots and nanorods in fields of 0.1–1.5 T.
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