Abstract
AbstractThe fluorination in gaseous phase of carbon tetrachloride has been investigated on aluminium fluoride with the aim of defining the mechanism of the reaction on this catalyst.The reactor and the operating conditions, were chosen in such a way as to isolate the effects of diffusion analysing the single reaction steps.While for the process in liquid phase the kinetics appears to be controlled by the formation of activated complexes between carbon tetrachloride and the catalytic support, the selective adsorption of HF on the catalyst is more probably the controlling step when the reaction is carried out in gaseous phase.
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