Flow characteristics in a horizontal reactor for continuous preparation of carbon nanotubes

Abstract

This study focuses on a sophisticated horizontal reactor designed to facilitate the continuous growth of carbon nanotubes (CNTs) through chemical vapor deposition (CVD). Experimental observations reveal that carbon production varies at different locations within the reactor, with higher yields typically found in the middle and rear zones. The flow dynamics within the reactor play a pivotal role in CNT growth, prompting a detailed simulation of the flow field using Computational Fluid Dynamics (CFD). This simulation leverages fluid dynamics principles to assess the impact of various parameters on the flow field, ultimately identifying the optimal operating conditions. Findings indicate that temperature-induced density contrasts create cyclic flow patterns that can negatively affect CNT growth rates. However, the gas flow inside the horizontal continuous preparation reactor can be improved and optimized by adjusting and controlling the preparation parameters. Appropriately lowering the heating temperature and the mole fraction of propylene in inlet 2, within the range of conditions suitable for the growth of CNTs, while minimizing the perturbation of the flow field by the shape of the carriers, can promote more favorable CNTs growth.