Abstract
Highly-transient free radicals may be identified positively in solution using fast electron spin resonance (esr) techniques, in experiments which also disclose the spin multiplicity of their precursor through the chemically-induced dynamic electron polarization (CIDEP) phenomenon. One form of CIDEP originates in the electron spin-correlated radical pair, an essential but largely unrecognised intermediate in radical reactions. The esr of this species itself can be observed in viscous or micellar solutions, or it can be observed using radical-yield detected magnetic resonance (RYDMR).
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