Fission of Hg*180,182,183 and Pt*178 nuclei at intermediate excitation energies

Abstract

Background: The nature of asymmetric fission of preactinides is not yet understood in detail, despite intense experimental and theoretical studies carried out at present.Purpose: The study of asymmetric and symmetric fission of $^{180,182,183}\mathrm{Hg}$ and $^{178}\mathrm{Pt}$ nuclei as a function of their excitation energy and isospin.Methods: Mass-energy distributions of fission fragments of $^{180}\mathrm{Hg}, ^{178}\mathrm{Pt}$ (two protons less than $^{180}\mathrm{Hg}$), and $^{182}\mathrm{Hg}$ (two neutrons more than $^{180}\mathrm{Hg}$) formed in the $^{36}\mathrm{Ar}+^{144}\mathrm{Sm}, ^{142}\mathrm{Nd}$, and $^{40}\mathrm{Ca}+^{142}\mathrm{Nd}$ reactions were measured at energies near and above the Coulomb barrier. Fission of $^{183}\mathrm{Hg}$ obtained in the reaction of $^{40}\mathrm{Ca}$ with $^{143}\mathrm{Nd}$ was also investigated to see if one extra neutron could lead to dramatic changes in the fission process due to the shape-staggering effect in radii, known in $^{183}\mathrm{Hg}$.The measurements were performed with the double-arm time-of-flight spectrometer CORSET.Results: The observed peculiarities in the fission fragment mass-energy distributions for all studied nuclei may be explained by the presence of a symmetric fission mode and three asymmetric fission modes, manifested by the different total kinetic energies and fragment mass splits. The yield of symmetric mode grows with increasing excitation energy of compound nucleus.Conclusions: The investigated properties of asymmetric fission of $^{180,182,183}\mathrm{Hg}$ and $^{178}\mathrm{Pt}$ nuclei point out the existence of well-deformed proton shell at $Z\ensuremath{\approx}36$ and a less deformed proton shell at $Z$ \ensuremath{\approx} 46.