Abstract

An applicable use of density functional theory (DFT) along with nonequilibrium Green's function (NEGF) is done for exploring the temperature-dependent spin electron transport nature in a ferromagnetic tungsten disulfide (WS2) nanoribbon. To demonstrate the effect of temperature on spin filtration and spin Seebeck effect, we evaluated vital parameters such as spin-polarized current and spin filtration efficiency. Spin filtration efficiency of around ∼95% is obtained in the high-temperature difference range. The high temperature (TL) of the left electrode in comparison to the high temperature (TR) of the right electrode results in higher and lower spin filtration efficiency in parallel magnetization (PM) and antiparallel magnetization (APM), respectively. Transmission spectrum plots at equilibrium are also calculated in PM and APM to justify the temperature-dependent spin transport behavior in the WS2 nanoribbon. Giant thermal magnetoresistance around 1.934 × 103% is achieved. The temperature-dependent negative differential resistance behavior of the current plot has been observed. Huge value of thermal magnetoresistance (MR) and excellent spin filtration obtained for WS2 nanoribbon suggests the potential application of this material in spin caloritronic devices.

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