Fingerprinting sources of beach sands by grain-size, using mid-infrared spectroscopy (MIRS) and portable XRF. Implications for coastal recovery along a tsunami-struck delta coastline

Abstract

Determining modern sediment provenance along sandy beaches helps understanding coastline dynamics and can therefore assist coastal management. Provenance analysis relies usually on mineralogical, elemental, and isotopic fingerprinting of sediment sources. Mid-Infrared Spectroscopy (MIRS) offers a rapid and non-destructive alternative. It relies on the identification of molecular-bonds in organic and inorganic materials. Thus far, MIRS has been used to fingerprint fine-grained sediments in mountainous and agricultural catchments. Here we use MIRS to analyze a range of sediment grain sizes (<0.25 mm; 0.25–0.5 mm; 0.5–2 mm) in modern fluvial and coastal sands, located in the delta of the Aceh River in Sumatra. Variations in molecular bond associations are compared to variations in major element concentration, quantified by portable X-ray fluorescence (pXRF) on a subset of samples. Covariations between MIRS and pXRF data are used to predict major element concentrations in all samples. Discriminant Analysis (DA) is used to classify sand-feeding streams into groups possessing distinctive MIRS fingerprints. DA proximity relationships are then used to predict the contribution of each source group to trunk stream sand and beach sands. The best discrimination is obtained among sands belonging to the medium grain-size fraction. Simple forward modeling of the expected contributions of the different sources is used to shade light on the DA-predicted association patterns. It helps discussing the biases introduced by sediment compositional changes from the headwaters to the coast, especially hydrodynamic sorting. We find that sand composition along the delta shoreline is primarily controlled by the asymmetric dispersal of sediment from the Aceh River mouth, owing to directional longshore drift. Local variations are generated by particle-size effects and by the propensity of the coast to erode or thicken over the past century. The coastal stretches the most severely damaged by the 2004 Indian Ocean Tsunami exhibit the greatest variations in apparent provenance between sub-fractions.