Fine-Tuning of the Magnetic Fano Resonance in Hybrid Oligomers via fs-Laser-Induced Reshaping

Abstract

Various clusters of metallic or dielectric nanoparticles can exhibit sharp Fano resonances originating from at least two modes interference of different spectral width. However, for practical applications such as biosensing or nonlinear nanophotonics, the fine-tuning of the Fano resonances is generally required. Here, we propose and demonstrate a novel type of hybrid oligomers consisting of asymmetric metal-dielectric (Au/Si) nanoparticles with a sharp Fano resonance in the visible range, which has a predominantly magnetic origin. We demonstrate both numerically and experimentally that such hybrid nanoparticle oligomers allow fine-tuning of the Fano resonance via fs-laser-induced melting of Au nanoparticles at the nanometer scale. We show that the Fano resonance wavelength can be changed by fs-laser reshaping very precisely (within 15 nm) being accompanied by a reconfiguration of its profile.