Abstract

Magnetic topological materials have attracted significant attention due to their potential realization of a variety of novel quantum phenomena. ${\mathrm{EuIn}}_{2}{\mathrm{As}}_{2}$ has recently been theoretically recognized as a long-awaited intrinsic antiferromagnetic bulk axion insulator. However, experimental studies of the transport properties arising from the topological states in this material are scarce. In this paper, we perform detailed magnetoresistance (MR) and Hall measurements to study the magnetotransport properties of this material. We find that the transport is strongly influenced by the spin configuration of the Eu moments from the concomitant change in the field dependence of the MR and that of the magnetization below the N\'eel temperature. Most importantly, an anomalous Hall effect (AHE) and a large topological Hall effect (THE) are observed. We suggest that the AHE is originated from a nonvanishing net Berry curvature due to the helical spin structure and that the THE is attributed to the formation of a noncoplanar spin texture with a finite scalar spin chirality induced by the external magnetic field in ${\mathrm{EuIn}}_{2}{\mathrm{As}}_{2}$. Our studies provide a platform to understand the influence of the interplay between the topology of electronic bands and the field-induced magnetic structure on magnetoelectric transport properties. In addition, our observations give a hint to realize axion insulator states and higher-order topological insulator states through manipulating the magnetic state of ${\mathrm{EuIn}}_{2}{\mathrm{As}}_{2}$.

Highlights

  • The success of topological band theory places studies of topological quantum states among the frontier topics in condensed matter physics in the last decades [1–4]

  • We suggest that the anomalous Hall effect (AHE) is originated from a nonvanishing net Berry curvature due to the helical spin structure and that the topological Hall effect (THE) is attributed to the formation of a noncoplanar spin texture with a finite scalar spin chirality induced by the external magnetic field in EuIn2As2

  • Our detailed transport measurements on bulk EuIn2As2 single crystals reveal that the transport properties in this compound are strongly influenced by the spin texture formed below TN

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Summary

INTRODUCTION

The success of topological band theory places studies of topological quantum states among the frontier topics in condensed matter physics in the last decades [1–4]. A real-space Berry phase arising from a skyrmion phase or a noncollinear spin texture with nonzero scalar spin chirality [χs = Si · (S j × Sk ) = 0, where Si, S j, and Sk are the three nearest spins] can act as a fictitious magnetic field on the conduction electrons, giving rise to the topological Hall effect (THE) [12–15]. A higher-order topological insulator phase with chiral hinge states is predicted with out-of-plane magnetic order [17]. These different topological states expected in the different orientations of the Eu moments provide a promising way to control the topological state by the external magnetic field. From the field and the angle dependence of the THE, we suggest that the THE is attributed to a finite χs caused by the noncoplanar spin texture formed under the out-of-plane magnetic field

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