Abstract

Electrical spin switching in an antiferromagnet is one of the key issues for both academic interest and industrial demand in new-type spin devices because an antiferromagnetic system has a negligible stray field due to an alternating sign between sub-lattices, in contrast to a ferromagnetic system. Naturally, questions arise regarding how fast and, simultaneously, how robustly the magnetization can be switched by external stimuli, e.g., magnetic field and spin current. First, the exploitation of ultrafast precessional motion of magnetization in antiferromagnetic oxide has been studied intensively. Regarding robustness, the so-called inertia-driven switching scenario has been generally accepted as the switching mechanism in antiferromagnet system. However, in order to understand the switching dynamics in a canted antiferromagnet, excited by magnetic field, accurate equation of motion and corresponding interpretation are necessary. Here, we re-investigate the inertia-driven switching process, triggered by the strict phase matching between effective driving field, dh/dt, and antiferromagnetic order parameters, l. Such theoretical approaches make it possible to observe the static parameters of an antiferromagnet, hosting Dzyaloshinskii–Moriya (DM) interaction. Indeed, we estimate successfully static parameters, such as DM, exchange, and anisotropy energies, from dynamical behaviour in YFeO3, studied using terahertz time-domain spectroscopy.

Highlights

  • In free-induction decay regime, we demonstrate in both experiment and theory that the precessional ellipticity in Sigma mode (S-mode), one of two resonant modes[24], provides

  • We investigate the field-driven dynamics of a canted antiferromagnet in both theory and experiment

  • In a free-induction decay regime, we found that the precessional ellipticity of S-mode determines DM energy in a canted antiferromagnet system

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Summary

Results and Discussion

The spin wave (or emission wave) perpendicular to the incident magnetic field is significantly dependent on the magnetization state[40] To remove this effect, we saturated magnetization by applying hz,DC. If spin waves are excited by the electric field of THz pulse, the experimental results that Faraday rotation signals in NiO12 and emission amplitudes in YFeO315 are linearly proportional to the pump field would be conjectured to be linear magneto-electric effect. Such coupling is not allowed in centrosymmetric system[45]

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