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Abstract
Spin dynamic of regio-regular Poly(3-octylthiophene-2,5-diyl) has been investigated with longitudinal field (LF) muon-spin-relaxation (μSR) techniques. The LF dependent muon-spin depolarization rate indicates the occurrence of dimensional crossover from one-dimensional intra-chain spin diffusion to three-dimensional inter-chain spin diffusion at 50 K.
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