Abstract
The infrared absorption spectra of CF 4 and CCl 4 have been observed in both the pure form and in rare gas matrices at low temperatures. The region studied corresponded to the ν 3, 2ν 4, and ν 3, ν 1+ν 4 Fermi doublets of CF 4 and CCl 4 respectively. The interaction of the vibrations in Fermi resonance in these molecules changes considerably from that found in the gaseous phase. The spectral features observed are discussed and related to S trizhevskii's theory.
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