Abstract
We have performed the fs pump–probe experiment on the B̃→ã nonadiabatic transition in the Hg–CO vdW complex. It is found that the transition occurs near the point where Hg and CO come nearest to each other on the B̃-state surface with a probability of 0.07 for their single encounter. This experiment serves as the first observation of the wave packet dynamics associated with an intermolecular energy flow in the vdW interaction.
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