Fast generation of cat states in Kerr nonlinear resonators via optimal adiabatic control

In this thesis we experimentally investigate quantum nonlocality: entangled states of spatially separated objects. Entanglement is one of the most striking consequences of the quantum formalism developed in the 1920's; the predicted outcomes of independent measurements on entangled objects reveal strong correlations that cannot be explained by classical physics. Early on, such predictions led physicists to doubt the validity and completeness of quantum theory. At the same time, entanglement is a key resource for applications in quantum information processing and a pre-requisite for many tasks in quantum communication and computation. This thesis attempts to answer two application driven questions: Firstly, can we generate useful entangled states of solid state spins for applications in quantum information processing? Secondly, can we use such entangled states as a resource to teleport an unknown quantum state? Finally, we ask a foundational question: Are our entangled states indeed inconsistent with the classical notions of free choice, locality and realism? Can we prove this experimentally, under the minimal assumptions of a loophole-free Bell test? To answer these questions we use single spins in ultra-pure diamonds. In particular, we use the electronic and nuclear spins associated with single nitrogen-vacancy (NV) defects. The NV centre is a point defect in diamond, consisting of a substitutional nitrogen (N) atom and a neighbouring missing carbon atom (vacancy, V). The NV centre possesses bound electronic states, whose energy levels lie well within the bandgap of the diamond host and whose spin degree of freedom can be used as a quantum bit (qubit). Because of the large diamond bandgap and the 99% spin free carbon-12 environment, the electronic spin qubit has exceptional coherence properties even at room temperature. Optical and microwave fields allow control of the electronic spin, which in turn allows control of nearby nuclear spins (the host nitrogen nuclear spin, and nearby carbon-13 spins). At liquid helium temperatures, spin-preserving optical transitions provide a powerful optical interface to the electronic spin, allowing, for example, projective readout of the spin state. By employing a protocol where entanglement is heralded by the detection of a single photon from each of two NV centres in diamonds separated by three metres, we find we can answer the first question in the affirmative. We show for the first time heralded entanglement between solid state quantum systems separated by a human-scale distance. Then, by combining the heralded entanglement with a deterministic local Bell state measurement and fast feed-forward, we show for the first time unconditional quantum teleportation over human-scale distances. We teleport an unknown quantum state from a nuclear spin in one diamond to an electronic spin in a diamond three meters away. Finally, by employing techniques from the previous experiments, we implement the first loophole-free Bell test. We separate two diamonds by 1.3 kilometres and optimize all operational fidelities, collection efficiencies and rates. This allows us to generate heralded entanglement between them approximately once an hour. The distance provides us with time to read out the electronic spin state in each diamond, faster than any lightlike signal could travel between them. The high-fidelity entangled state preparation and spin readout are sufficient to violate the Clauser-Horne-Shimony-Holt Bell-inequality. Combined with fast random number generators and a robust statistical analysis, we find a significant rejection of the local-realist hypothesis, without requiring additional experimental assumptions. The results in this thesis open the door to various applications in quantum information processing. In particular, a remote photonic entangling operation may enable future quantum networks. In such a network the nodes would be formed by the NV centre's combined electronic and nuclear spin register. The nodes would be linked by photonic entanglement operations. Such a network could be used for long distance secure communication, provide a connection between separated quantum computers, or form the basis of a fault tolerant quantum computer by itself. Furthermore, a loophole-free Bell test demonstrates the possibility to do device independent randomness generation and key distribution, that could form the basis for future secure communication channels.

Photonic cat states stored in high-Q resonators show great promise for hardware efficient universal quantum computing. We propose an approach to efficiently prepare such cat states in a Kerr-nonlinear resonator by the use of a two-photon drive. Significantly, we show that this preparation is robust against single-photon loss. An outcome of this observation is that a two-photon drive can eliminate undesirable phase evolution induced by a Kerr nonlinearity. By exploiting the concept of transitionless quantum driving, we moreover demonstrate how non-adiabatic initialization of cat states is possible. Finally, we present a universal set of quantum logical gates that can be performed on the engineered eigenspace of such a two-photon driven resonator and discuss a possible realization using superconducting circuits. The robustness of the engineered subspace to higher-order circuit nonlinearities makes this implementation favorable for scalable quantum computation.

Superposition of two coherent states, the Schrodinger’s cat state, can exhibit different nonclassical properties having foundational applications in quantum information processing. We consider the ‘superposition of Schrodinger’s cat state with the vacuum state (SCVS)’ of the optical field. We discuss different witness of nonclassicality properties such as lower- and higher-order squeezing (viz., squeezing, Hong & Mandel’s fourth-order squeezing, amplitude-squared squeezing) and sub-Poissonian photon statistics. Further, we discuss the negativity of the Wigner function of SCVS indicating the nonclassicality of the state under investigation. We find that the vacuum state contribution in SCVS exhibits different nonclassicalities under some conditions stronger where the nonclassicalities exhibited by the state without vacuum state contribution are weaker.

A single photon source which generates transform limited single photons is highly desirable for applications in quantum optics. Transform limited emission guarantees the indistinguishability of the emitted single photons. This, in turn brings groundbreaking applications in linear optics quantum information processing within an experimental reach. Recently, self-assembled InAs quantum dots and trapped atoms have successfully been demonstrated as such sources for highly indistinguishable single photons. Here, we demonstrate that nearly transform limited zero-phonon-line (ZPL) emission from single molecules can be obtained by using vibronic excitation. Furthermore we report the results of coincidence detection experiments at the output of a Michelson-type interferometer. These experiments reveal Hong-Ou-Mandel correlations as a proof of the indistinguishability of the single photons emitted consecutively from a single molecule. Therefore, single molecules constitute an attractive alternative to single InAs quantum dots and trapped atoms for applications in linear optics quantum information processing. Experiments were performed with a home-built confocal microscope keeping the sample in a superfluid liquid Helium bath at 1.4K. We investigated terrylenediimide (TDI) molecules highly diluted in hexadecane (Shpol'skii matrix). A continuous wave single mode dye laser was used for excitation of vibronic transitions of individual molecules. From the integral fluorescence, the ZPL of single molecules was selected with a spectrally narrow interference filter. The ZPL emission was then sent to a scanning Fabry-Perot interferometer for linewidth measurements or a Michelson-type interferometer for coincidence detection.

We show that by engineering the interaction with the environment there exists a large class of systems that can evolve irreversibly to a cat state. To be precise we show that it is possible to engineer an irreversible process so that the steady state is close to a pure Schrödinger’s cat state by using double well systems and an environment comprising two-photon (or phonon) absorbers. We also show that it should be possible to prolong the lifetime of a Schrödinger’s cat state exposed to the destructive effects of a conventional single-photon decohering environment. In addition to our general analysis we present a concrete circuit realisation of both system and environment that should be fabricatable with current technologies. Our protocol should make it easier to prepare and maintain Schrödinger cat states which would be useful in applications of quantum metrology and information processing as well as being of interest to those probing the quantum to classical transition.

Entanglement is a fundamental resource for various optical quantum information processing (QIP) applications. To achieve high-speed QIP systems, entanglement should be encoded in short wavepackets. Here we report the real-time observation of ultrafast optical Einstein–Podolsky–Rosen correlation at a picosecond timescale in a continuous-wave system. Optical phase-sensitive amplification using a 6-THz-bandwidth waveguide-based optical parametric amplifier enhances the effective efficiency of 70-GHz-bandwidth homodyne detectors, mainly used in 5G telecommunication, enabling its use in real-time quantum state measurement. Although power measurement using frequency scanning, such as an optical spectrum analyser, is not performed in real time, our observation is demonstrated through the real-time amplitude measurement and can be directly used in QIP applications. The observed Einstein–Podolsky–Rosen states show quantum correlation of 4.5 dB below the shot-noise level encoded in wavepackets with 40 ps period, equivalent to 25 GHz repetition—103 times faster than previous entanglement observation in continuous-wave systems. The quantum correlation of 4.5 dB is already sufficient for several QIP applications, and our system can be readily extended to large-scale entanglement. Moreover, our scheme has high compatibility with optical communication technology such as wavelength-division multiplexing, and femtosecond-timescale observation is also feasible. Our demonstration is a paradigm shift in accelerating accessible quantum correlation—the foundational resource of all quantum applications—from the nanosecond to picosecond timescales, enabling ultrafast optical QIP.

We determine the evolving probability representation of entangled cat states in the potential of either the harmonic oscillator or the inverted oscillator, assuming that the states are initially prepared in the potential of the harmonic oscillator. Such states have several applications in quantum information processing. The inverted quantum harmonic oscillator, where the potential energy corresponds to imaginary frequencies of the oscillator, can be applied in relation to cosmological problems. We also determine the evolving probability representation of cat states of an oscillating spin-1/2 particle of the inverted oscillator, in which the time evolution of the spin state is described by an arbitrary unitary operator. The properties of the determined entangled probability distributions are discussed.

We propose a feasible experimental model to investigate the generation and characterization of nonclassical states in a cavity optomagnonic system consisting of a ferromagnetic YIG sphere that simultaneously supports both the magnon mode and two whispering gallery modes of optical photons. The photons undergo the magnon-induced Brillouin light scattering, which is a well-established tool for the cavity-assisted manipulations of magnons as well as magnon spintronics. At first, we derive the desired interaction Hamiltonian under the influence of the anti-Stokes scattering process and then proceed to analyze the dynamical evolution of quantum statistics of photons and magnons as well as their intermodal entanglement. The results show that both photons and magnons generally acquire some nonclassical features, e.g., the strong antibunching and anti-correlation. Interestingly, the system may experience the perfect photon and magnon blockade phenomena, simultaneously. Besides, the nonclassical features may be protected against the unwanted environmental effects for a relatively long time, especially, in the weak driving field regime and when the system is initiated with a small number of particles. However, it should be noted that some fast quantum-classical transitions may occur in-between. Although the unwanted dissipative effects plague the nonclassical features, we show that this system can be adopted to prepare optomagnonic entangled states. The generation of entangled states depends on the initial state of the system and the interaction regime. The intermodal photon-magnon entanglement may be generated and pronounced, especially, if the system is initialized with low intensity even Schrödinger cat state in the strong coupling regime. The cavity-assisted manipulation of magnons is a unique and flexible mechanism that allows an interesting test bed for investigating the interdisciplinary contexts involving quantum optics and spintronics. Moreover, such a hybrid optomagnonic system may be used to design both on-demand single-photon and single-magnon sources and may find potential applications in quantum information processing.

Among the classes of highly entangled states of multiple quantum systems, the so-called 'Schrödinger cat' states are particularly useful. Cat states are equal superpositions of two maximally different quantum states. They are a fundamental resource in fault-tolerant quantum computing and quantum communication, where they can enable protocols such as open-destination teleportation and secret sharing. They play a role in fundamental tests of quantum mechanics and enable improved signal-to-noise ratios in interferometry. Cat states are very sensitive to decoherence, and as a result their preparation is challenging and can serve as a demonstration of good quantum control. Here we report the creation of cat states of up to six atomic qubits. Each qubit's state space is defined by two hyperfine ground states of a beryllium ion; the cat state corresponds to an entangled equal superposition of all the atoms in one hyperfine state and all atoms in the other hyperfine state. In our experiments, the cat states are prepared in a three-step process, irrespective of the number of entangled atoms. Together with entangled states of a different class created in Innsbruck, this work represents the current state-of-the-art for large entangled states in any qubit system.

Quantum state transfer (QST) and entangled state generation (ESG) are\nimportant building blocks for modern quantum information processing. To achieve\nthese tasks, convention wisdom is to consult the quantum adiabatic evolution,\nwhich is time-consuming, and thus is of low fidelity. Here, using the shortcut\nto adiabaticity technique, we propose a general method to realize high-fidelity\nfast QST and ESG in a cavity-coupled many qubits system via its dark pathways,\nwhich can be further designed for high-fidelity quantum tasks with different\noptimization purpose. Specifically, with a proper dark pathway, QST and ESG\nbetween any two qubits can be achieved without decoupling the others, which\nsimplifies experimental demonstrations. Meanwhile, ESG among all qubits can\nalso be realized in a single step. In addition, our scheme can be implemented\nin many quantum systems, and we illustrate its implementation on\nsuperconducting quantum circuits. Therefore, we propose a powerful strategy for\nselective quantum manipulation, which is promising in cavity coupled quantum\nsystems and could find many convenient applications in quantum information\nprocessing.\n

Superradiance and subradiance concerning enhanced and inhibited collective radiation of an ensemble of atoms have been a central topic in quantum optics. However, precise generation and control of these states remain challenging. Here we deterministically generate up to 10-qubit superradiant and 8-qubit subradiant states, each containing a single excitation, in a superconducting quantum circuit with multiple qubits interconnected by a cavity resonator. The sqrt[N]-scaling enhancement of the coupling strength between the superradiant states and the cavity is validated. By applying an appropriate phase gate on each qubit, we are able to switch the single collective excitation between superradiant and subradiant states. While the subradiant states containing a single excitation are forbidden from emitting photons, we demonstrate that they can still absorb photons from the resonator. However, for an even number of qubits, a singlet state with half of the qubits being excited can neither emit nor absorb photons, which is verified with 4 qubits. This study is a step forward in coherent control of collective radiation and has promising applications in quantum information processing.

We present a new hardware-efficient paradigm for universal quantum computation which is based on encoding, protecting and manipulating quantum information in a quantum harmonic oscillator. This proposal exploits multi-photon driven dissipative processes to encode quantum information in logical bases composed of Schrödinger cat states. More precisely, we consider two schemes. In a first scheme, a two-photon driven dissipative process is used to stabilize a logical qubit basis of two-component Schrödinger cat states. While such a scheme ensures a protection of the logical qubit against the photon dephasing errors, the prominent error channel of single-photon loss induces bit-flip type errors that cannot be corrected. Therefore, we consider a second scheme based on a four-photon driven dissipative process which leads to the choice of four-component Schrödinger cat states as the logical qubit. Such a logical qubit can be protected against single-photon loss by continuous photon number parity measurements. Next, applying some specific Hamiltonians, we provide a set of universal quantum gates on the encoded qubits of each of the two schemes. In particular, we illustrate how these operations can be rendered fault-tolerant with respect to various decoherence channels of participating quantum systems. Finally, we also propose experimental schemes based on quantum superconducting circuits and inspired by methods used in Josephson parametric amplification, which should allow one to achieve these driven dissipative processes along with the Hamiltonians ensuring the universal operations in an efficient manner.

Harmonic oscillators count among the most fundamental quantum systems with important applications in molecular physics, nanoparticle trapping, and quantum information processing. Their equidistant energy level spacing is often a desired feature, but at the same time a challenge if the goal is to deterministically populate specific eigenstates. Here, we show how interference in the transition amplitudes in a bichromatic laser field can suppress the sequential climbing of harmonic oscillator states (Kapitza-Dirac blockade) and achieve selective excitation of energy eigenstates, cat states, and other non-Gaussian states. This technique can transform the harmonic oscillator into a coherent two-level system or be used to build a large-momentum-transfer beam splitter for matter waves. To illustrate the universality of the concept, we discuss feasible experiments that cover many orders of magnitude in mass, from single electrons over large molecules to dielectric nanoparticles.

Quantum hyperentanglement and its applications in quantum information processing

Vortex solitons (VSs) in spin-orbit-coupled (SOC) quantum gases are of fundamental interest due to their unique topological properties and potential applications in quantum information processing. We investigate the existence and stability of two-dimensional (2D) matter-wave VSs in a binary SOC Bose-Einstein condensate (BEC) of Rydberg atoms, confined by a radially periodic potential. By employing the imaginary-time integration method, we numerically demonstrate the formation of three distinct types of matter-wave soliton pairs, ring-shaped, necklace-shaped, and crescent-shaped, carrying topological charges up to 7. Their stability is systematically verified through temporal evolution and fidelity analysis. The SOC strength is found to be critical for supporting VSs with high topological charges. However, the presence of the external potential imposes a constraint on the SOC interaction, suppressing the generation of VSs with very high charges. A repulsive Rydberg-Rydberg interaction is identified as essential for balancing the diffraction and the SOC effect. Furthermore, the phase structures of these solitons exhibit a periodic modulation in the radial direction, inherited from the external potential. This study provides significant promise for applications in quantum information processing and the design of novel topological devices.