Abstract
As an important sustainable energy source, Li-ion batteries have been widely used in mobile phones, electric vehicles, large-scale energy storage and aerospace. However, due to the inevitable safety risks of traditional liquid Li-ion batteries, the use of all-solid-state batteries to replace organic liquid electrolytes has become one of the most effective ways to solve safety problem. Solid-state electrolyte (SSE) is the core part of all-solid-state Li-ion battery. The ideal solid-state electrolyte has the characteristics of high ionic conductivity, wide enough electrochemical stability window, suitable mechanical strength and excellent chemical stability. In particular, high ionic conductivity is an essential prerequisite. While, so far only a few solid-state electrolytes exhibit the Li ionic conductivities higher than 10−4 S/cm at room temperature.
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