Abstract
In recent years, significant development milestones have been reached in the areas of facilitated transport membranes and ionic liquids for CO2 separations, making the combination of these materials an incredibly promising technology platform for gas treatment processes, such as post-combustion and direct CO2 capture from air in buildings, submarines, and spacecraft. The developments in facilitated transport membranes involve consistently surpassing the Robeson upper bound for dense polymer membranes, demonstrating a high CO2 flux across the membrane while maintaining very high selectivity. This mini review focuses on the recent developments of facilitated transport membranes, in particular discussing the challenges and opportunities associated with the incorporation of ionic liquids as fixed and mobile carriers for separations of CO2 at low partial pressures (<1 atm).
Highlights
Facilitated Transport MembranesSignificant development milestones have been reached in the areas of facilitated transport membranes and ionic liquids for CO2 separations, making the combination of these materials an incredibly promising technology platform for gas treatment processes, such as post-combustion and direct CO2 capture from air in buildings, submarines, and spacecraft
To reduce CO2 emissions and mitigate the adverse effects of CO2-induced climate change (Ballantyne et al, 2018), removal of CO2, from atmosphere (Siriwardane et al, 2005) and pre-/postprocess streams (Chen et al, 2012; Chen and Ho, 2016), has been a focus of research
These gel-type facilitated transport membranes (FTMs) cannot be fabricated into stand-alone films due to the fragility of the gel, so a porous support or secondary gel network is used for mechanical support
Summary
Significant development milestones have been reached in the areas of facilitated transport membranes and ionic liquids for CO2 separations, making the combination of these materials an incredibly promising technology platform for gas treatment processes, such as post-combustion and direct CO2 capture from air in buildings, submarines, and spacecraft. The developments in facilitated transport membranes involve consistently surpassing the Robeson upper bound for dense polymer membranes, demonstrating a high CO2 flux across the membrane while maintaining very high selectivity. This mini review focuses on the recent developments of facilitated transport membranes, in particular discussing the challenges and opportunities associated with the incorporation of ionic liquids as fixed and mobile carriers for separations of CO2 at low partial pressures (
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