Abstract
To remove multitudinous pollutants from wastewater, the design of a highly efficient and multifunctional photocatalyst is necessary. A novel CQDs/SnO2-x/BiOI photocatalyst (named CSnBI composite) was prepared by combining carbon quantum dots (CQDs), large specific surface area SnO2-x nanocrystals and BiOI nanocrystals to obtain a compact hybrid structure. TEM and Raman techniques confirmed the structure of CSnBI composite. The photocurrent and EIS showed that the photoexcited electron-hole pairs separation efficiency was improved. As anticipated, novel CSnBI photocatalyst can successfully remove tetracycline, methyl orange, E. coli (Escherichia coli) and S. aureus under a LED light due to the hybridization contaction among CQDs, SnO2-x and BiOI. The mechanism showed that the introduction of CQDs promoted visible light absorption and efficient separation of photogenerated carriers of SnO2-x/BiOI heterojunction. The capture experiment and related measurements showed that h+, •O2- and •OH are active species in the photocatalytic process. This study gave a novel case for facile construction of photocatalysts with tight hybrid structure.
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