Abstract
Graphene-based composite aerogel (GCA) refers to a solid porous substance formed by graphene or its derivatives, graphene oxide (GO) and reduced graphene oxide (rGO), with inorganic materials and polymers. Because GCA has super-high adsorption, separation, electrical properties, and sensitivity, it has great potential for application in super-strong adsorption and separation materials, long-life fast-charging batteries, and flexible sensing materials. GCA has become a research hotspot, and many research papers and achievements have emerged in recent years. Therefore, the fabrication, structure, performance, and application prospects of GCA are summarized and discussed in this review. Meanwhile, the existing problems and development trends of GCA are also introduced so that more will know about it and be interested in researching it.
Highlights
The research results indicate that Graphene-based composite aerogel (GCA) has lower density, higher porosity, smaller pore diameter, larger specific surface area, and more stable morphology compared to general aerogels, but more importantly it has some unique characteristics, such as higher heat resistance, better electrical conductivity, and higher absorbability of metal ions [2,3]
We focus on several types of GCA, including graphene-based/2D nanomaterial (MXenes) aerogel for sensors and supercapacitors, graphene-based/inorganic nanomaterial (SiO2, SnO2, SnO2, TiO2 ) aerogel and heat-insulating flame-retardant materials, and graphene-based/synthetic polymer aerogel and graphene-/natural sugar-based polymer aerogel used as adsorbents to remove metal ions and dye contaminants in water
This paper describes the influence of differences in the morphological structure of GCA on its mechanical, thermal, and electrochemical properties
Summary
A highly porous material with low density and high specific surface area, is obtained by replacing the liquid in wet gel with gas without significantly changing the structure and volume of the gel network. Its functions are mainly derived from graphene and its derivatives (graphene-based materials), while its structure and volume stability are mainly determined by other matrix materials [1]. The research results indicate that GCA has lower density, higher porosity, smaller pore diameter, larger specific surface area, and more stable morphology compared to general aerogels, but more importantly it has some unique characteristics, such as higher heat resistance, better electrical conductivity, and higher absorbability of metal ions [2,3]. (b) multi-layer graphene, (c) GO, (d) rGO [6]
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