Abstract
We report a facile chemical method for fabricating holey graphene by catalytic oxidation of highly ordered pyrolytic graphite (HOPG) using an FeIII porphyrin complex-based covalent organic framework (COF) as a bifunctional surface catalyst-template. We demonstrate regular hole formation after oxidation with H2 O2 and NaOCl, COF removal, and HOPG exfoliation.
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