Extinction of buoyant turbulent non-premixed flames under reduced oxygen concentrations

Abstract

Local and global extinction of 10 kW buoyant turbulent non-premixed flames of methane from a 13.7 cm diameter burner under oxygen concentrations (OCs) from 20.9 % to 12 % are investigated using a combination of OH* chemiluminescence imaging and exhaust-gas sampling. Local flame extinction, indicated by holes or discontinuities in the OH* images, is only observed at OC lower than 17 %. For OC below 16 %, large-scale turbulent flow dynamics causes rapid creation of large extinction holes that do not reclose, and the overall combustion efficiency (η) decreases rapidly as local extinction becomes more probable. Direct observation of local extinction in buoyant turbulent flames provides important physical insights and validation data for models of extinction and re-ignition by distinguishing their respective contributions to η. We observe that local extinction events are associated with large-scale flow features, leading us to hypothesize that extinction behavior correlates with resolved-scale strain rates from large-eddy simulation (LES) in excess of the laminar extinction limit. This idea is investigated by performing LES for the target flame, extracting strain-rate statistics on the flame surface, and comparing these to both the extinction limits for canonical counterflow diffusion flames and to the experimentally observed extinction behavior. Results show that the cumulative distribution of turbulent flame strain rates up to the laminar extinction limit closely follows the measured OC dependence of η. This approach to η works well for different OCs and other fuels such as propane and ethylene, which suggests great potential for the development of computationally efficient extinction models for fire suppression.