Explosive growth characteristics of 5.6–560 nm particles and deposition in human respiratory during spring in Yangtze River Delta region, China

Abstract

Studying the contribution of regional transport to ultrafine particles (UFPs) and the deposition effect of nanoscale particles in human respiratory system is conducive to exploring the impact of atmospheric particles on the environment and human health. Based on the data set of number concentration spectrum in the particle size range of 5.6–560 nm in the spring of Hefei, the Yangtze River Delta region obtained by a fast mobility particle sizer, the explosive growth characteristics, potential source identification and deposition flux analysis of UFPs were systematically studied. The results showed that the frequency of new particle formation (NPF) events during spring was 31.5 %. SO2 and O3 contribute to NPF events. Daytime, higher temperature, stronger solar radiation and lower humidity were more conducive to the explosive growth of UFPs. In addition, regional transport of pollutants from the cities around Hefei played an important role in the accumulation mode particles, which were mainly affected by the land-source air mass from northwest Jiangsu (23.64 %) and the sea-source air mass from the Yellow Sea (23.99 %). It was worth noting that approximately 10,406 ng of UFPs enters the human respiratory system every day. The main deposition area of 5.6–560 nm nanoscale particles was alveolar, 5.6–400 nm is more likely to be deposited on alveolar, while nanoscale particles with particle size between 400 and 560 nm is more likely to be deposited on head airways. This study identified the deposition risk of nanoscale particles in the respiratory system under different particle sizes.