Abstract

We numerically study the jamming transition of frictionless polydisperse spheres in three dimensions. We use an efficient thermalisation algorithm for the equilibrium hard sphere fluid and generate amorphous jammed packings over a range of critical jamming densities that is about three times broader than in previous studies. This allows us to reexamine a wide range of structural properties characterizing the jamming transition. Both isostaticity and the critical behavior of the pair correlation function hold over the entire range of jamming densities. At intermediate length scales, we find a weak, smooth increase of bond orientational order. By contrast, distorted icosahedral structures grow rapidly with increasing the volume fraction in both fluid and jammed states. Surprisingly, at large scale we observe that denser jammed states show stronger deviations from hyperuniformity, suggesting that the enhanced amorphous ordering inherited from the equilibrium fluid competes with, rather than enhances, hyperuniformity. Finally, finite size fluctuations of the critical jamming density are considerably suppressed in the denser jammed states, indicating an important change in the topography of the potential energy landscape. By considerably stretching the amplitude of the critical “J-line”, our work disentangles physical properties at the contact scale that are associated with jamming criticality, from those occurring at larger length scales, which have a different nature.

Highlights

  • We numerically study the jamming transition of frictionless polydisperse spheres in three dimensions

  • Panel (b) demonstrates instead that above the onset volume fraction, φonset 0.56, around which glassy dynamics starts to manifest in the equilibrium fluid [79], the equilibrium fluid and the corresponding jammed states are characterized by very similar bond orientational order; at the local scale, jammed configurations retain essentially the local structure of the parent fluid

  • Thanks to an efficient thermalisation algorithm which allowed us to equilibrate polydisperse hard spheres up to unprecedented packing fractions [44], we have significantly extended the study of the line of critical jamming transitions, or J-line

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Summary

Introduction

Granular materials such as grains, pinballs, and large colloids flow when some external forces are applied. It has been reported that systems prepared at the jamming transition have unexpected density fluctuations at large scales, possibly corresponding to hyperuniform behavior. We can characterize the variation of structural properties with φJ over an unprecedentedly broad range of volume fractions, φJ ≈ 0.65 − 0.70 This range is at least 3 times wider than in any previous study of frictionless jammed packings [31, 40].

The model
Equilibration of very dense fluid states
Compression towards the jamming transition
Extending the range of jamming densities
Isostaticity
Pair correlation function at contact
Structure at the large scale
Findings
Discussion and conclusions
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