Abstract

Redox reactions between fine solid fuels, such as pulverized coal powder, and coarse oxygen carrier particles can be carried out in a fixed/moving bed reactor chemical looping system. The migration pattern of the solid fuel powder and its contact time with coarse particles can significantly affect the reaction rate and the product yield. A number of challenges exist in transporting/mixing of fuel powder and in removing noncombustible waste (e.g., coal ash) from the reactor vessel in the chemical looping operation. Thus, it is important to understand the hydrodynamic behaviors of fine particles in such situations. This study describes an experimental approach that examines migration characteristics of fine particles (Geldart A/B), in both spatial and temporal aspects, in a packed bed of coarse particles (Geldart D). The experimental variables include the particle size distribution of the fine powder, the fine to coarse mass ratio, and flow conditions. At a given upward aeration flow within the range that i...

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