Abstract

Abstract. In order to gain understanding on the vertical structure of atmospheric water vapour above mountain lakes and to assess its link with the isotopic composition of the lake water and with small-scale dynamics (i.e. valley winds, thermal convection above complex terrain), the L-WAIVE (Lacustrine-Water vApor Isotope inVentory Experiment) field campaign was conducted in the Annecy valley in the French Alps during 10 d in June 2019. This field campaign was based on an original experimental synergy between a suite of ground-based, boat-borne, and two ultra-light aircraft (ULA) measuring platforms implemented to characterize the thermodynamic and isotopic composition above and in the lake. A cavity ring-down spectrometer and an in-cloud liquid water collector were deployed aboard one of the ULA to characterize the vertical distribution of the main stable water isotopes (H216O, H218O and H2H16O) both in the air and in shallow cumulus clouds. The temporal evolution of the meteorological structures of the low troposphere was derived from an airborne Rayleigh–Mie lidar (embarked on a second ULA), a ground-based Raman lidar, and a wind lidar. ULA flight patterns were repeated several times per day to capture the diurnal evolution as well as the variability associated with the different weather events encountered during the field campaign, which influenced the humidity field, cloud conditions, and slope wind regimes in the valley. In parallel, throughout the campaign, liquid water samples of rain, at the air–lake water interface, and at 2 m depth in the lake were taken. A significant variability of the isotopic composition was observed along time, depending on weather conditions, linked to the transition from the valley boundary layer towards the free troposphere, the valley wind intensity, and the vertical thermal stability. Thus, significant gradients of isotopic content have been revealed at the transition to the free troposphere, at altitudes between 2.5 and 3.5 km. The influence of the lake on the atmosphere isotopic composition is difficult to isolate from other contributions, especially in the presence of thermal instabilities and valley winds. Nevertheless, such an effect appears to be detectable in a layer of about 300 m thickness above the lake in light wind conditions. We also noted similar isotopic compositions in cloud drops and rainwater.

Highlights

  • Why are the vertical structures of the stable isotope of the water vapour field in the lower troposphere only sparsely documented above Alpine lakes? This is in part due to the complexity and fast-evolving nature of the low-level atmospheric circulation in Alpine-type valleys which is intimately

  • Since the experiment was conducted in a valley, where ERA5 reanalyses are generally considered not to be very accurate below the average altitude of the mountains (∼ 2 km a.m.s.l. in our case), it is more informative to use the measurements acquired during the field campaign from the lidar and ultra-light aircraft (ULA) to describe the evolution of meteorological variables

  • The L-WAIVE field campaign documented for the first-time vertical profiles of stable water isotopes over an Alpine lake valley, in combination with lidar and meteorological measurements

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Summary

Introduction

Why are the vertical structures of the stable isotope of the water vapour field in the lower troposphere only sparsely documented above Alpine lakes? This is in part due to the complexity and fast-evolving nature of the low-level atmospheric circulation in Alpine-type valleys which is intimately. Why are the vertical structures of the stable isotope of the water vapour field in the lower troposphere only sparsely documented above Alpine lakes? The link between hydrology and evaporation has mainly been investigated using vapour and liquid water isotopes measurements gathered just above the Earth’s surface and samples from lake water and precipitation Unexploited potential remains in using stable water isotopes to increase our understanding of the influence of evaporation, boundary-layer processes, and the free troposphere for local and regional climate conditions in Alpine lakes. For this purpose, we have implemented an original multiplatform experimental approach based on continuous highresolution vertical profiling of tropospheric water vapour, temperature, and wind, as well as scattering layers (aerosols, clouds) in the valley.

L-WAIVE experimental strategy
Measurement platforms
Deployment
Airborne payloads
ULA-IC
Ground-based instrumentation
Raman lidar
Wind lidar
Boat-borne payload: lake and atmospheric sampling
Precipitation sampling
Synoptic conditions
Insight on the local atmospheric conditions derived from lidars
Water vapour isotope during L-WAIVE
Atmospheric in situ sampling
Cloud liquid water sampling
Precipitation liquid water isotope composition
Lake liquid water isotope composition
Synthesis and discussion
Vertical profiles in the low troposphere as observed from ULA
Statistical overview of isotopic content from the lake to the atmosphere
Conclusion
Processing of liquid samples for stable water isotope analysis
Findings
Processing of stable isotope measurements in water vapour
Sensitivity of CRDS instrument parameters to flight conditions

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