Abstract

Hydrogen safety is a primary obstacle to the widespread use of hydrogen energy, and the risk of hydrogen utilization can be avoided by eliminating unnecessary hydrogen immediately. Here we report a new kind of hydrogen elimination catalyst based on ZrVFe hydrogen storage alloy supported Pt. The chemical reduction temperature and the Pt loading have a great influence on the hydrogen elimination performance. When the reduction temperature is 60 °C and the Pt loading is 2 wt%, the ZrVFe/Pt catalyst exhibits excellent hydrogen elimination ability at 2–20 vol% hydrogen concentration, especially the efficiency of hydrogen elimination at 20 vol% hydrogen concentration is as high as 99%. The hydrogen adsorption capacity of the ZrVFe/Pt catalyst was 13 times higher than that of the commonly used metal carrier FeCrAl/Pt catalyst. This work paves a new direction for the design and on-going development of hydrogen elimination catalyst for hydrogen energy applications.

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