Experimental investigation of mesoscopic heterogeneous motion of laser-activated self-propelling Janus particles in suspension.

Abstract

The mesoscopic collective motion of self-propelling active particle suspension is experimentally investigated. The active particles are silica micro spheres with Au hemisphere coating, and their propelling strength is activated by laser irradiation. The suspension is driven from equilibrium to near equilibrium and far from equilibrium by tuning the excitation laser intensity. By use of the long-term particle tracking technique, the time evolution of a large amount of active particles is resolvable. For low laser intensity, the suspension is driven to near equilibrium state with homogeneous superdiffusion motion. The strength of enhanced superdiffusion is monotonically related to the laser intensity. For high laser intensity, the motility-induced phase separation with the coexistence of dense cluster and very dilute individual particle are observed. It leads to highly heterogeneous dynamic with less mobile jammed cluster and fast-moving particles and subsequently suppresses the enhanced superdiffusion. Such heterogeneous dynamics is similar to many far from equilibrium systems. Finally, the degree away from equilibrium (Gaussian dynamics) triggered by propelling strength is quantified by non-Gaussian parameters.