Abstract

A single crystal of potassium dihydrogen phosphate (KH2PO4, KDP), which possesses unique excellent non-linear electro-optical properties, is currently the only material suitable for electro-optic switches and high power laser-frequency conversion applications in laser-induced inertial confinement fusion. However, KDP crystals are difficult to produce because of their inherent softness, brittleness, and water-solubility, as well as their strong anisotropy and temperature sensitivity. Obtaining high-quality near-lossless KDP elements is an issue that should be solved urgently. In this study, an ultra-precision numerical control polishing method based on the water dissolution principle was introduced to achieve a controllable material removal. A small polishing tool was used to process a large KDP surface, and an accurate tool influence functions is required for deterministic fabrication of KDP surface. In order to quantify the influence of critical parameters (e.g., polishing speed, polishing pressure, water content, and directions of revolution and rotation) on material removal rate distribution, a tool influence function model was established based on the Preston equation. The model was then modified based on experiments, and its accuracy was verified. This modified model lays the foundation for ultra-precision water dissolution polishing of large KDP crystals. A very smoothed surface with high surface accuracy (peak-to-valley value below 0.4 λ) and low surface roughness (Ra 1.598 nm) could indeed be obtained by using the model. This research is also applicable to the polishing of other water-soluble materials.

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