Experimental determination of phase transitions by means of configurational entropies in finite Yukawa balls.

Abstract

The phase transition of finite Yukawa balls (ordered systems of microspheres in a gaseous plasma environment) with less than 100 particles is studied experimentally by means of configurational entropies. We have developed cylindrical two- and three-particle-correlation functions to measure these entropies for multiple cluster sizes over a wide temperature range. The cluster temperature is finely tuned using a stochastic laser heating setup. It is shown that the correlation functions give a detailed insight into the structural properties of the cluster. The derived configurational entropies give a clear indication of the transition temperature from a solid-like to a fluid-like state. Comparing the transition temperatures of different sized clusters it is found that the transition temperature increases with cluster size in general agreement with theoretical predictions.