Abstract

Microbottle resonators (MBR) have attracted research interest for studying nonlinear optical interactions in last two decades, due to the ultra-tight optical confinement in spaces of three dimensions. In this paper, silica MBRs exhibiting rich resonant modes with ultra-high quality factor up to <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math notation="LaTeX">$3.73 \times {10^8}$</tex-math></inline-formula> are demonstrated, based on which a portable and robust packaged platform with a tapered fiber coupling is established. Such a packaged platform effectively avoids external perturbations such as air flow and tiny mechanical vibrations, which supports our experimental demonstration of nonlinear scattering effects including four-wave mixing (FWM), simulated Raman scattering, and simulated Brillouin scattering. As a result, Raman-assisted FWM and Brillouin-assisted FWM are observed due to the strong field enhancement in the MBR. In a further investigation, a Kerr frequency comb with broad bandwidth of ∼200 nm and a Raman-assisted comb with a bandwidth up to ∼50 nm is achieved, correspondingly. Our works show the versatility of MBR for fundamental research and may open a new route to the development of practical applications in frequency conversion, spectroscopy and communications.

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