Abstract

Strong molecule-light interaction enables the control of molecular structures and dynamical processes. A model with strong laser drive is proposed to greatly enhance the intermolecular distance of resonant energy transfer, where the molecules are strongly driven by an optical cavity. The optimal Rabi frequency and quantum yield of energy transfer are observed, resulting from the trade off between dipole-dipole interaction and molecule-cavity coupling. When the strong drive at certain Rabi frequency is applied, a larger spatial range of effective energy transfer and a slower decay rate with the distance compared to the F\"orster mechanism of resonant energy transfer are observed in our model. Our work sheds light on spectroscopic study of the cooperative energy transfer in molecular polaritons.

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.