Abstract

The quantum world distinguishes itself from the classical world by being governed by probability amplitudes rather than probabilities. On a single-particle level, quantum phases can be manipulated leading to observable interference patterns that can be used as a probe e.g. in matter wave microscopy. But the quantum world bears even more fascinating effects when it comes to the interplay between more than one particle. Correlations between quantum particles such as entanglement can be exploited to speed up computational algorithms or enable secure cryptography. Here, we propose and numerically explore a thought experiment to address the question whether quantum correlations between particles can be used in matter wave microscopy. Specifically, we address the following questions: can information be transferred between two mutually spin-correlated free-electron wavepackets? Can Coulomb and exchange correlations be linked to the decoherence and dephasing mechanisms of matter waves? Using a time-dependent Hartree–Fock algorithm, we will show that the exchange term has a substantial role in transferring the information between two mutually spin-correlated electrons, whereas the Hartree potential (or mean-field Coulomb potential) dominates the dephasing on a single-particle level. Our findings might facilitate fermionic matter wave interferometry experiments designed to retrieve information about non-classical correlations and the mechanism of decoherence in open quantum systems.

Highlights

  • In contrast to classical probability distributions, quantum probabilities are determined by probability amplitudes

  • On a single-particle level, quantum phases can be manipulated leading to observable interference patterns that can be used as a probe e.g. in matter wave microscopy

  • We address the following questions: Can information be transferred between two mutually spin-correlated free-electron wavepackets? Can Coulomb and exchange correlations be linked to the decoherence and dephasing mechanisms of matter waves? Using a time-dependent Hartree-Fock algorithm, we will show that the exchange term has a substantial role in transferring the information between two mutually spincorrelated electrons, whereas the Hartree potential dominates the dephasing on a single-particle level

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Summary

Introduction

In contrast to classical probability distributions, quantum probabilities are determined by probability amplitudes. The ability to coherently manipulate the phase of a quantum object with holograms or laser light, and to detect it, has revolutionized the world of matter-wave interferometry [1, 2] and microscopy [3]. The ability to coherently manipulate the phase of a free-electron wavepacket using near-field optical distributions in the vicinity of nano-objects has been manifested by Zewail and coworkers [8], pioneering the field of photon-induced near-field electron microscopy (PINEM) [9]. In addition to PINEM, coherent manipulation of the electron phase by transverse light in free space due to nonlinear processes caused by the ponderomotive interaction [17, 18] paves the way for on-demand electron-wave shaping and might be used for phase-contrast microscopy

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