Abstract

In this work, various tunable sized spinel ferrite MnFe2O4 nanoparticles (namely MF20, MF40, MF60 and MF80) with reduced graphene oxide (RGO) were embedded in a polypropylene (PP) matrix. The particle size and structural feature of magnetic filler MnFe2O4 nanoparticles were controlled by sonochemical synthesis time 20 min, 40 min, 60 min and 80 min. As a result, the electromagnetic interference shielding characteristics of developed nanocomposites MF20-RGO-PP, MF40-RGO-PP, MF60-RGO-PP and MF80-RGO-PP were also controlled by tuning of magnetic/dielectric loss. The maximum value of total shielding effectiveness (SET) was 71.3 dB for the MF80-RGO-PP nanocomposite sample with a thickness of 0.5 mm in the frequency range (8.2–12.4 GHz). This lightweight, flexible and thin nanocomposite sheet based on the appropriate size of MnFe2O4 nanoparticles with reduced graphene oxide demonstrates a high-performance advanced nanocomposite for cutting-edge electromagnetic interference shielding application.

Highlights

  • Extensive practice of electronic and communication devices, liberating electromagnetic (EM) waves, generates EM radiation pollution [1]

  • The particle size and structural feature of magnetic filler MnFe2O4 nanoparticles were controlled by sonochemical synthesis time 20 min, 40 min, 60 min and 80 min

  • The electromagnetic interference shielding characteristics of developed nanocomposites MF20-reduced graphene oxide (RGO)-PP, MF40-RGO-PP, MF60-RGO-PP and MF80-RGO-PP were controlled by tuning of magnetic/dielectric loss

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Summary

Introduction

Extensive practice of electronic and communication devices, liberating electromagnetic (EM) waves, generates EM radiation pollution [1]. Electromagnetic interference (EMI) does affect the working and life of electronic devices and is harmful to human health [2]. This noble type of EM radiation pollution delivers a solid motivation to develop efficient EMI shielding materials [3]. Lightweight, thinness and cost efficiency are other additional necessities of high-performance EMI shielding materials for operational applications [4]. Polymer-based EMI shielding composite materials are lightweight, resistant to corrosion, flexible and simple in preparation [5]. The performance of polymer-based EMI shielding materials depends on the intrinsic electrical conductivity, aspect ratio, and concentration of the fillers [6]. Spinel ferrite nanoparticles as nanofillers have been established as potential magnetic absorbers due to their outstanding magnetic loss, good stability and cost-effectiveness [8,9]

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