Ex-situ quantification of impurity deposition depth on HL-2A divertor graphite tile by laser-induced breakdown spectroscopy

Abstract

During tokamak discharges, the Plasma Wall Interaction (PWI) would lead to impurity deposition and fuel retention on the surface of the Plasma Facing Materials (PFMs). Laser-induced breakdown spectroscopy (LIBS) has emerged as a promising technique to facilitate in-situ, real-time, online characterization of the impurity deposition and fuel retention on the wall of tokamaks for PWI studies. The purpose of this investigation is to quantify the impurity deposition layer on the graphite tile removed from the dome region of the HL-2A tokamak lower divertor by using the ex-situ LIBS approach. The investigations indicate that the primarily deposited impurity elements are Fe, Cr, Ni, Mn, Ca, Al, Cu, Si, C, which may originate from the stainless steel first wall, divertor, limiter or the siliconized wall conditioning due to the PWI process in HL-2A tokamak. This has been further supported by observing a significantly positive correlation between the Cr, Ni, Mn, Al and Fe elements by spectral cumulative intensity linear regression analysis. The 3D morphology of the laser-ablated craters is reconstructed using a confocal microscope, revealing the laser ablation rates for the deposition layer and the substrate graphite tile to be 348 nm/pulse and 220 nm/pulse, respectively, under the laser fluence of 10 J/cm2. Then the thickness of the deposition layer is determined by using the correlation coefficient method. Along the poloidal direction of HL-2A tokamak, the deposited impurity shows an inhomogeneous pattern, with the thickness of the deposition layer varying from 1.74 μm to 5.92 μm. Finally, the absolute depth distribution of each element is also quantitatively measured.