Abstract

We report on low-temperature heat-transport properties of the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuCl$_4$. Broad maxima in the thermal conductivity along the three principal axes, observed at about 5 K, are interpreted in terms of the Debye model, including the phonon Umklapp scattering. For thermal transport along the $b$ axis, we observed a pronounced field-dependent anomaly, close to the transition into the three-dimensional long-range-ordered state. No such anomalies were found for the transport along the $a$ and $c$ directions. We argue that this anisotropic behavior is related to an additional heat-transport channel through magnetic excitations, that can best propagate along the direction of the largest exchange interaction. Besides, peculiarities of the heat transport of Cs$_2$CuCl$_4$ in magnetic fields up to the saturation field and above are discussed.

Highlights

  • We report on low-temperature heat-transport properties of the spin-1/2 triangular-lattice antiferromagnet Cs2CuCl4

  • We argue that this anisotropic behavior is related to an additional heat-transport channel through magnetic excitations, that can best propagate along the direction of the largest exchange interaction

  • Spin-1/2 Heisenberg antiferromagnets (AFs) on triangular lattices have attracted particular attention, representing an important class of lowdimensional frustrated magnets and allowing one to probe effects of the geometrical frustration, magnetic order, and quantum fluctuations in strongly correlated spin systems. This interest was stimulated by the idea of the “resonating valence bond” (RVB) ground state for an AF system of spins on a triangular layer lattice [7]

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Summary

Introduction

Evidence of one-dimensional magnetic heat transport in the triangular-lattice antiferromagnet Cs2CuCl4 We report on low-temperature heat-transport properties of the spin-1/2 triangular-lattice antiferromagnet Cs2CuCl4. For thermal transport along the b axis, we found a pronounced field-dependent anomaly, close to the transition into the three-dimensional long-range-ordered state.

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