Abstract
Evidence is presented for a local interaction between CO and Na adsorbed onRu(001). For low coverages of Na(θ Na ⪅ 0.15 ML) and saturation coverages of CO at 80 K, a fraction of the CO molecules undergo a substantial change in bonding configuration: molecular CO bound perpendicular to the Ru(001) surface changes to an “inclined” configuration in the presence of low coverages of Na.
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