Evaluation of the Effects of Particle Characteristics on the Terminal Settling Velocities of Microplastics in Stagnant Waters using CFD

Abstract

<p>Mismanaged waste leads to inputs of microplastics into the environment and the aquatic system affecting rivers and lakes. The physical properties of microplastic (MP) particles affect their terminal settling velocity (TSV) in the water column and in turn their distribution patterns in aquatic systems. To evaluate the settling behavior and the TSV of MP particles we simulated the settling of a large range of MP particles with regular and irregular shapes in the water column using a computational fluid dynamics (CFD) model. To validate the results returned by our model, we compared CFD findings to the corresponding results obtained by semi-empirical relationships as well as the results from experiments for 120 irregularly shaped MP particles with sizes and densities ranging from 500 to 2000 µm and 1.03 to 1.38 grcm<sup>-3</sup>, respectively. The CFD results are in good agreement with the results from the laboratory and semi-empirical relationships with a 0.05 difference in the slopes of their linear regressions. In a next step, we defined scenarios to systematically investigate the influence of different particle characteristics such as roundness, density, and volume as well as water temperature on the TSV of regular and irregular MP particles. Our simulations revealed a dominant effect of particle density on the TSV compared to the effects of the other parameters. For example, doubling particle densities increased the TSVs of the MP particles up to 500%, while, doubling their volumes only led to a maximum increase in their TSV of 200%. Increasing the roundness of the MP particles, letting them evolve towards a perfect sphere, increased their TSVs by up to 15%, while seasonal changes in lake water temperatures typical for lakes in temperate climate regions, caused changes in TSVs by up to 32%.</p>