Abstract
This study proposed to use barite-enhanced ultra-high performance geopolymer concrete (UHPGC) as the composite matrix to develop high-strength, cement-free, and sustainable radiation shielding materials. The physical properties, γ ray attenuation capacity, microstructure, and environmental and economic impacts of prepared barite-enhanced radiation shielding UHPGC were determined and compared with normal concrete and ultra-high performance concrete (UHPC). The combination of steel fibers and barite aggregate increased the density of UHPGC, thereby enhancing its γ ray attenuation capacity. Multi-scale γ ray shielding simulation results demonstrated that although thickness was the more decisive factor of γ ray attenuation capacity of composites, the enhancement of the shielding capacity of the material helps reduce the floor area and the cost of radiation shielding structure. The micro-analysis results revealed that barite-enhanced UHPGC exhibited compact microstructure and excellent interfacial performance. Furthermore, life cycle assessment results demonstrated that UHPGC was more suitable as a composite matrix than UHPC to develop sustainable and low-cost radiation shielding materials.
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