Abstract
We measured conducting and magnetic properties of (ET)4[Ln(NCS)6]·CH2Cl2 (Ln = Dy, Ho, Er, and Yb), (ET)5[Ln(NCS)6NO3]·EtOH (Ln = Tb and Dy), and (TTF)6[Dy(NCS)6]. All of the complexes behaved as semiconductors irrespective of Ln ions used, and also exhibited anomalous frequency-dependence of ac magnetic susceptibility below ca. 10 K, especially for Dy derivatives, indicating blocking behavior as found in single-molecule magnets.
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