Estimation of the radon production rate in granite rocks and evaluation of the implications for geogenic radon potential maps: A case study in Central Portugal

Abstract

The goal of this study was to estimate radon gas production rate in granitic rocks and identify the factors responsible for the observed variability. For this purpose, 180 samples were collected from pre-Hercynian and Hercynian rocks in north and central Portugal and analysed for a) 226Ra activity, b) radon (222Rn) per unit mass activity, and c) radon gas emanation coefficient. On a subset of representative samples from the same rock types were also measured d) apparent porosity and e) apparent density. For each of these variables, the values ranged as follows: a) 15 to 587Bqkg-1, b) 2 to 73Bqkg-1, c) 0.01 to 0.80, d) 0.3 to 11.4 % and e) 2530 to 2850kgm-3. Radon production rate varied between 40 to 1386Bqm-3h-1. The variability observed was associated with geologically late processes of low and high temperature which led to the alteration of the granitic rock with mobilization of U and increase in radon 222Rn gas emanation. It is suggested that, when developing geogenic radon potential maps, data on uranium concentration in soils/altered rock should be used, rather than data obtained from unaltered rock.