Abstract
Abstract. Open biomass burning (OBB) has significant impacts on air pollution, climate change and potential human health. OBB has gathered wide attention but with little focus on the annual variation of pollutant emission. Central and eastern China (CEC) is one of the most polluted regions in China. This study aims to provide a state-of-the-art estimation of the pollutant emissions from OBB in CEC from 2003 to 2015, by adopting the satellite observation dataset – the burned area product (MCD64Al) and the active fire product (MCD14 ML) – along with local biomass data (updated biomass loading data and high-resolution vegetation data) and local emission factors. The successful adoption of the double satellite dataset for long-term estimation of pollutants from OBB with a high spatial resolution can support the assessing of OBB on regional air quality, especially for harvest periods or dry seasons. It is also useful to evaluate the effects of annual OBB management policies in different regions. Here, monthly emissions of pollutants were estimated and allocated into a 1×1 km spatial grid for four types of OBB including grassland, shrubland, forest and cropland. From 2003 to 2015, the emissions from forest, shrubland and grassland fire burning had an annual fluctuation, whereas the emissions from crop straw burning steadily increased. The cumulative emissions of organic carbon (OC), elemental carbon (EC), methane (CH4), nitric oxide (NOx), non-methane volatile organic compounds (NMVOCs), sulfur dioxide (SO2), ammonia (NH3), carbon monoxide (CO), carbon dioxide (CO2) and fine particles (PM2.5) were 3.64×103, 2.87×102, 3.05×103, 1.82×103, 6.4×103, 2.12×102, 4.67×102, 4.59×104, 9.39×105 and 4.13×103 Gg in these years, respectively. Crop straw burning was the largest contributor for all pollutant emissions, by 84 %–96 %. For the forest, shrubland and grassland fire burning, forest fire burning emissions contributed the most, and emissions from grassland fire were negligible due to little grass coverage in this region. High pollutant emissions concentrated in the connection area of Shandong, Henan, Jiangsu and Anhui, with emission intensity higher than 100 tons per square kilometer, which was related to the frequent agricultural activities in these regions. Peak emission of pollutants occurred during summer and autumn harvest periods including May, June, September and October, during which ∼50 % of the total pollutant emissions were emitted in these months. This study highlights the importance of controlling the crop straw burning emissions. From December to March, the crop residue burning emissions decreased, while the emissions from forest, shrubland and grassland exhibited their highest values, leading to another small peak in emissions of pollutants. Obvious regional differences in seasonal variations of OBB were observed due to different local biomass types and environmental conditions. Rural population, agricultural output, economic levels, local burning habits, social customs and management policies were all influencing factors for OBB emissions.
Highlights
Open biomass burning (OBB), which includes forest, shrubland, grassland and crop residue fire burning, is one of the most important sources for gaseous and particulate matter (PM) especially for fine particulate particles (PM2.5) and associated carbonaceous aerosols (Zha, 2013; Yan et al, 2014; Zong et al, 2016; Zhou et al, 2017)
J =1 where j stands the different aggregated vegetation types; i stands for different pollutant species; Ei,x,t is the emission amount of pollutant i in location x and month t; BAx,t is the total burned area of aggregated vegetation class in location x and month t; CEx is defined as the combustion efficiency in location x; BLx is the biomass fuel loading in location x; EFi,j is the emission factor of pollutant specie i for vegetation type j
A combination of the burned area product (MCD64Al) with the active fire product (MCD14 ML), as well as local high-resolution vegetation speciation data, updated local biomass data, local emission factors and survey results were used to estimate the pollutant emissions from open burning in Central and eastern China (CEC) from 2003 to 2015
Summary
Open biomass burning (OBB), which includes forest, shrubland, grassland and crop residue fire burning (van der Werf et al, 2010; Qiu et al, 2016), is one of the most important sources for gaseous and particulate matter (PM) especially for fine particulate particles (PM2.5) and associated carbonaceous aerosols (elemental carbon, EC; organic carbon, OC) (Zha, 2013; Yan et al, 2014; Zong et al, 2016; Zhou et al, 2017). The pollutants with high emission amounts from OBB posed significant impacts on regional and global climate change, air quality and human health Former studies have highlighted the role of OBB on worsening air quality regionally or in megacities, especially for crop residue burning during harvest periods (Yamaji et al, 2010; Zhu et al, 2010; Huang et al, 2012b; Su et al, 2012; Cheng et al, 2014; Zhou et al, 2016; Zhang et al, 2017)
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