Abstract
An ESR investigation has been made on the first intrinsically conducting LB films consisting of the charge transfer complex, TMTTF-octadecylTCNQ. The occurrence of a single line without structures and observed g value indicate that there is a strong coupling between TMTTF radical spins and TCNQ radical spins as in the TTF-TCNQ crystal. The temperature dependence of the spin susceptibility of the system implies the presence of spin species due to conduction electrons, which is consistent with the conductivity measurements.
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