Abstract
The entropy theory of binary liquid mixture was extended to include the excess configurational entropy SCE, which reflects the degree of structural change on mixing. The SCE values were obtained for several hydrocarbon-hydrocarbon, alcohol-alcohol and amine-alcohol systems from their mole-fraction dependence of the glass transition temperatures and precise heat capacity data of the pure components. The liquid structures of the systems, especially those related to the formation of the hydrogen bonds, are discussed based on SCE.
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