Abstract
The enthalpy values associated with solid—solid interactions of uranyl nitrate with both urea and thiourea to form mixed complexes are studied. The tendency of the urea to substitute the thiourea molecules bonded with the uranyl ion was observed. A greater facility of the ligand (hard or soft) to coordinate with the UO 2+ 2 ion in those complexes in which a greater number of ligand molecules are present was found.
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