Enhancing off-axis integrated cavity output spectroscopy (OA-ICOS) with radio frequency white noise for gas sensing.

Abstract

Injecting radio frequency (RF) white noise to the current driving of the laser can broaden the laser emission linewidth and efficiently suppress cavity-mode noise in off-axis integrated cavity output spectroscopy (OA-ICOS). The effect of the injected RF noise level on the cavity-mode noise and the deformation of the absorption line shape in off-axis integrated cavity output spectroscopy (OA-ICOS) with a distributed feedback laser (DFB) at 1.65 µm were investigated. We measured methane at different concentrations between 0.1 ppmv and 2 ppmv associated with a -20 dBm RF noise injection. A linear spectral response of the intensity of the cavity output spectra with the CH4 concentration was observed. A threefold improvement in the detection limit was achieved compared to unperturbed OA-ICOS. The response time of the improved OA-ICOS system is about 30 s and the minimum detectable concentration (MDC) of CH4 is 7.6 ppbv, which corresponds to a minimum detectable fractional absorption scaled to the path length of 7.3 × 10-10 cm-1. The noise equivalent absorption sensitivity of the system is 5.51 × 10-9 cm-1Hz-1/2.