Abstract

AbstractWe extend a stochastic aerosol‐snow albedo model to explicitly simulate dust internally/externally mixed with snow grains of different shapes and for the first time quantify the combined effects of dust‐snow internal mixing and snow nonsphericity on snow optical properties and albedo. Dust‐snow internal/external mixing significantly enhances snow single‐scattering coalbedo and absorption at wavelengths of <1.0 μm, with stronger enhancements for internal mixing (relative to external mixing) and higher dust concentrations but very weak dependence on snow size and shape variabilities. Compared with pure snow, dust‐snow internal mixing reduces snow albedo substantially at wavelengths of <1.0 μm, with stronger reductions for higher dust concentrations, larger snow sizes, and spherical (relative to nonspherical) snow shapes. Compared to internal mixing, dust‐snow external mixing generally shows similar spectral patterns of albedo reductions and effects of snow size and shape. However, relative to external mixing, dust‐snow internal mixing enhances the magnitude of albedo reductions by 10%–30% (10%–230%) at the visible (near‐infrared) band. This relative enhancement is stronger as snow grains become larger or nonspherical, with comparable influences from snow size and shape. Moreover, for dust‐snow external and internal mixing, nonspherical snow grains have up to ~45% weaker albedo reductions than spherical grains, depending on snow size, dust concentration, and wavelength. The interactive effect of dust‐snow mixing state and snow shape highlights the importance of accounting for these two factors concurrently in snow modeling. For application to land/climate models, we develop parameterizations for dust effects on snow optical properties and albedo with high accuracy.

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